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10.1038/ncomms15553 http://scihub22266oqcxt.onion/10.1038/ncomms15553 C5458515!5458515 !28541308     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=28541308 &cmd=llinks): Failed to open stream: HTTP request failed! 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The controlled disassembly of mesostructured perovskites as an avenue to fabricating high performance nanohybrid catalysts |pdf=|usr=}}{{28541308 }} gab.com Text The controlled disassembly of mesostructured perovskites as an avenue to fabricating high performance nanohybrid catalysts JO: Nat Commun http://www.kidney.de/pget.php?&tw=1&pmid=28541308 #FOAvip Versatile superstructures composed of nanoparticles have recently been prepared using various disassembly methods. However, little information is known on how the structural disassembly influences the catalytic performance of the materials. Here we show how the disassembly of an ordered porous La(0.6)Sr(0.4)MnO(3) perovskite array, to give hexapod mesostructured nanoparticles, exposes a new crystal facet which is more active for catalytic methane combustion. On fragmenting three-dimensionally ordered macroporous (3DOM) structures in a controlled manner, via a process that has been likened to retrosynthesis, hexapod-shaped building blocks can be harvested which possess a mesostructured architecture. The hexapod-shaped perovskite catalyst exhibits excellent low temperature methane oxidation activity (T(90%)=438?°C; reaction rate=4.84 × 10(-7)?mol?m(-2)?s(-1)). First principle calculations suggest the fractures, which occur at weak joints within the 3DOM architecture, afford a large area of (001) surface that displays a reduced energy barrier for hydrogen abstraction, thereby facilitating methane oxidation. Twit Text FOAVip The controlled disassembly of mesostructured perovskites as an avenue to fabricating high performance nanohybrid catalysts ????Nat Commun http://www.kidney.de/pget.php?&tw=1&pmid=28541308 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=28541308 #FOAvip English Wikipedia <ref>{{Cite pmid|28541308 }}</ref> The controlled disassembly of mesostructured perovskites as an avenue to fabricating high performance nanohybrid catalysts #MMPMID28541308 Wang Y ; Arandiyan H ; Tahini HA ; Scott J ; Tan X ; Dai H ; Gale JD ; Rohl AL ; Smith SC ; Amal R Nat Commun 2017[May]; 8 (ä): 15553 PMID28541308 show ga Versatile superstructures composed of nanoparticles have recently been prepared using various disassembly methods. However, little information is known on how the structural disassembly influences the catalytic performance of the materials. Here we show how the disassembly of an ordered porous La(0.6)Sr(0.4)MnO(3) perovskite array, to give hexapod mesostructured nanoparticles, exposes a new crystal facet which is more active for catalytic methane combustion. On fragmenting three-dimensionally ordered macroporous (3DOM) structures in a controlled manner, via a process that has been likened to retrosynthesis, hexapod-shaped building blocks can be harvested which possess a mesostructured architecture. The hexapod-shaped perovskite catalyst exhibits excellent low temperature methane oxidation activity (T(90%)=438?°C; reaction rate=4.84 × 10(-7)?mol?m(-2)?s(-1)). First principle calculations suggest the fractures, which occur at weak joints within the 3DOM architecture, afford a large area of (001) surface that displays a reduced energy barrier for hydrogen abstraction, thereby facilitating methane oxidation. äThe controlled disassembly of mesostructured perovskites as an avenue (epmc).pdf DeepDyve Pubget Overpricing