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10.1126/sciadv.1601659 http://scihub22266oqcxt.onion/10.1126/sciadv.1601659 C5384807!5384807 !28435874     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=28435874 &cmd=llinks): Failed to open stream: HTTP request failed! 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Toward garnet electrolyte-based Li metal batteries: An ultrathin, highly effective, artificial solid-state electrolyte/metallic Li interface |pdf=|usr=}}{{28435874 }} gab.com Text Toward garnet electrolyte-based Li metal batteries: An ultrathin, highly effective, artificial solid-state electrolyte/metallic Li interface JO: Sci Adv http://www.kidney.de/pget.php?&tw=1&pmid=28435874 #FOAvip Solid-state batteries are a promising option toward high energy and power densities due to the use of lithium (Li) metal as an anode. Among all solid electrolyte materials ranging from sulfides to oxides and oxynitrides, cubic garnet-type Li(7)La(3)Zr(2)O(12) (LLZO) ceramic electrolytes are superior candidates because of their high ionic conductivity (10(-3) to 10(-4) S/cm) and good stability against Li metal. However, garnet solid electrolytes generally have poor contact with Li metal, which causes high resistance and uneven current distribution at the interface. To address this challenge, we demonstrate a strategy to engineer the garnet solid electrolyte and the Li metal interface by forming an intermediary Li-metal alloy, which changes the wettability of the garnet surface (lithiophobic to lithiophilic) and reduces the interface resistance by more than an order of magnitude: 950 ohm·cm(2) for the pristine garnet/Li and 75 ohm·cm(2) for the surface-engineered garnet/Li. Li(7)La(2.75)Ca(0.25)Zr(1.75)Nb(0.25)O(12) (LLCZN) was selected as the solid-state electrolyte (SSE) in this work because of its low sintering temperature, stabilized cubic garnet phase, and high ionic conductivity. This low area-specific resistance enables a solid-state garnet SSE/Li metal configuration and promotes the development of a hybrid electrolyte system. The hybrid system uses the improved solid-state garnet SSE Li metal anode and a thin liquid electrolyte cathode interfacial layer. This work provides new ways to address the garnet SSE wetting issue against Li and get more stable cell performances based on the hybrid electrolyte system for Li-ion, Li-sulfur, and Li-oxygen batteries toward the next generation of Li metal batteries. Twit Text FOAVip Toward garnet electrolyte-based Li metal batteries: An ultrathin, highly effective, artificial solid-state electrolyte/metallic Li interface ????Sci Adv http://www.kidney.de/pget.php?&tw=1&pmid=28435874 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=28435874 #FOAvip English Wikipedia <ref>{{Cite pmid|28435874 }}</ref> Toward garnet electrolyte-based Li metal batteries: An ultrathin, highly effective, artificial solid-state electrolyte/metallic Li interface #MMPMID28435874 Fu KK ; Gong Y ; Liu B ; Zhu Y ; Xu S ; Yao Y ; Luo W ; Wang C ; Lacey SD ; Dai J ; Chen Y ; Mo Y ; Wachsman E ; Hu L Sci Adv 2017[Apr]; 3 (4 ): e1601659 PMID28435874 show ga Solid-state batteries are a promising option toward high energy and power densities due to the use of lithium (Li) metal as an anode. Among all solid electrolyte materials ranging from sulfides to oxides and oxynitrides, cubic garnet-type Li(7)La(3)Zr(2)O(12) (LLZO) ceramic electrolytes are superior candidates because of their high ionic conductivity (10(-3) to 10(-4) S/cm) and good stability against Li metal. However, garnet solid electrolytes generally have poor contact with Li metal, which causes high resistance and uneven current distribution at the interface. To address this challenge, we demonstrate a strategy to engineer the garnet solid electrolyte and the Li metal interface by forming an intermediary Li-metal alloy, which changes the wettability of the garnet surface (lithiophobic to lithiophilic) and reduces the interface resistance by more than an order of magnitude: 950 ohm·cm(2) for the pristine garnet/Li and 75 ohm·cm(2) for the surface-engineered garnet/Li. Li(7)La(2.75)Ca(0.25)Zr(1.75)Nb(0.25)O(12) (LLCZN) was selected as the solid-state electrolyte (SSE) in this work because of its low sintering temperature, stabilized cubic garnet phase, and high ionic conductivity. This low area-specific resistance enables a solid-state garnet SSE/Li metal configuration and promotes the development of a hybrid electrolyte system. The hybrid system uses the improved solid-state garnet SSE Li metal anode and a thin liquid electrolyte cathode interfacial layer. This work provides new ways to address the garnet SSE wetting issue against Li and get more stable cell performances based on the hybrid electrolyte system for Li-ion, Li-sulfur, and Li-oxygen batteries toward the next generation of Li metal batteries. äToward garnet electrolyte-based Li metal batteries: An ultrathin, high(epmc).pdf DeepDyve Pubget Overpricing