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10.3390/nano5010233 http://scihub22266oqcxt.onion/10.3390/nano5010233 C5312858!5312858 !28347008     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=28347008 &cmd=llinks): Failed to open stream: HTTP request failed! 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New Insights into Understanding Irreversible and Reversible Lithium Storage within SiOC and SiCN Ceramics |pdf=|usr=}}{{28347008 }} gab.com Text New Insights into Understanding Irreversible and Reversible Lithium Storage within SiOC and SiCN Ceramics JO: Nanomaterials (Basel) http://www.kidney.de/pget.php?&tw=1&pmid=28347008 #FOAvip Within this work we define structural properties of the silicon carbonitride (SiCN) and silicon oxycarbide (SiOC) ceramics which determine the reversible and irreversible lithium storage capacities, long cycling stability and define the major differences in the lithium storage in SiCN and SiOC. For both ceramics, we correlate the first cycle lithiation or delithiation capacity and cycling stability with the amount of SiCN/SiOC matrix or free carbon phase, respectively. The first cycle lithiation and delithiation capacities of SiOC materials do not depend on the amount of free carbon, while for SiCN the capacity increases with the amount of carbon to reach a threshold value at ~50% of carbon phase. Replacing oxygen with nitrogen renders the mixed bond Si-tetrahedra unable to sequester lithium. Lithium is more attracted by oxygen in the SiOC network due to the more ionic character of Si-O bonds. This brings about very high initial lithiation capacities, even at low carbon content. If oxygen is replaced by nitrogen, the ceramic network becomes less attractive for lithium ions due to the more covalent character of Si-N bonds and lower electron density on the nitrogen atom. This explains the significant difference in electrochemical behavior which is observed for carbon-poor SiCN and SiOC materials. Twit Text FOAVip New Insights into Understanding Irreversible and Reversible Lithium Storage within SiOC and SiCN Ceramics ????Nanomaterials (Basel) http://www.kidney.de/pget.php?&tw=1&pmid=28347008 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=28347008 #FOAvip English Wikipedia <ref>{{Cite pmid|28347008 }}</ref> New Insights into Understanding Irreversible and Reversible Lithium Storage within SiOC and SiCN Ceramics #MMPMID28347008 Graczyk-Zajac M ; Reinold LM ; Kaspar J ; Sasikumar PV ; Soraru GD ; Riedel R Nanomaterials (Basel) 2015[Feb]; 5 (1 ): 233-245 PMID28347008 show ga Within this work we define structural properties of the silicon carbonitride (SiCN) and silicon oxycarbide (SiOC) ceramics which determine the reversible and irreversible lithium storage capacities, long cycling stability and define the major differences in the lithium storage in SiCN and SiOC. For both ceramics, we correlate the first cycle lithiation or delithiation capacity and cycling stability with the amount of SiCN/SiOC matrix or free carbon phase, respectively. The first cycle lithiation and delithiation capacities of SiOC materials do not depend on the amount of free carbon, while for SiCN the capacity increases with the amount of carbon to reach a threshold value at ~50% of carbon phase. Replacing oxygen with nitrogen renders the mixed bond Si-tetrahedra unable to sequester lithium. Lithium is more attracted by oxygen in the SiOC network due to the more ionic character of Si-O bonds. This brings about very high initial lithiation capacities, even at low carbon content. If oxygen is replaced by nitrogen, the ceramic network becomes less attractive for lithium ions due to the more covalent character of Si-N bonds and lower electron density on the nitrogen atom. This explains the significant difference in electrochemical behavior which is observed for carbon-poor SiCN and SiOC materials. äNew Insights into Understanding Irreversible and Reversible Lithium St(epmc).pdf DeepDyve Pubget Overpricing