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10.1038/ncomms13278

http://scihub22266oqcxt.onion/10.1038/ncomms13278
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suck abstract from ncbi


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pmid27827360
      Nat+Commun 2016 ; 7 (ä): 13278
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  • Unusually efficient photocurrent extraction in monolayer van der Waals heterostructure by tunnelling through discretized barriers #MMPMID27827360
  • Yu WJ ; Vu QA ; Oh H ; Nam HG ; Zhou H ; Cha S ; Kim JY ; Carvalho A ; Jeong M ; Choi H ; Castro Neto AH ; Lee YH ; Duan X
  • Nat Commun 2016[Nov]; 7 (ä): 13278 PMID27827360 show ga
  • Two-dimensional layered transition-metal dichalcogenides have attracted considerable interest for their unique layer-number-dependent properties. In particular, vertical integration of these two-dimensional crystals to form van der Waals heterostructures can open up a new dimension for the design of functional electronic and optoelectronic devices. Here we report the layer-number-dependent photocurrent generation in graphene/MoS(2)/graphene heterostructures by creating a device with two distinct regions containing one-layer and seven-layer MoS(2) to exclude other extrinsic factors. Photoresponse studies reveal that photoresponsivity in one-layer MoS(2) is surprisingly higher than that in seven-layer MoS(2) by seven times. Spectral-dependent studies further show that the internal quantum efficiency in one-layer MoS(2) can reach a maximum of 65%, far higher than the 7% in seven-layer MoS(2). Our theoretical modelling shows that asymmetric potential barriers in the top and bottom interfaces of the graphene/one-layer MoS(2)/graphene heterojunction enable asymmetric carrier tunnelling, to generate usually high photoresponsivity in one-layer MoS(2) device.
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