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10.1038/ncomms13169 http://scihub22266oqcxt.onion/10.1038/ncomms13169 C5105156!5105156 !27827376     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=27827376 &cmd=llinks): Failed to open stream: HTTP request failed! 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A metal-organic cage incorporating multiple light harvesting and catalytic centres for photochemical hydrogen production |pdf=|usr=}}{{27827376 }} gab.com Text A metal-organic cage incorporating multiple light harvesting and catalytic centres for photochemical hydrogen production JO: Nat Commun http://www.kidney.de/pget.php?&tw=1&pmid=27827376 #FOAvip Photocatalytic water splitting is a natural but challenging chemical way of harnessing renewable solar power to generate clean hydrogen energy. Here we report a potential hydrogen-evolving photochemical molecular device based on a self-assembled ruthenium-palladium heterometallic coordination cage, incorporating multiple photo- and catalytic metal centres. The photophysical properties are investigated by absorption/emission spectroscopy, electrochemical measurements and preliminary DFT calculations and the stepwise electron transfer processes from ruthenium-photocentres to catalytic palladium-centres is probed by ultrafast transient absorption spectroscopy. The photocatalytic hydrogen production assessments reveal an initial reaction rate of 380??mol?h(-1) and a turnover number of 635 after 48?h. The efficient hydrogen production may derive from the directional electron transfers through multiple channels owing to proper organization of the photo- and catalytic multi-units within the octahedral cage, which may open a new door to design photochemical molecular devices with well-organized metallosupramolecules for homogenous photocatalytic applications. Twit Text FOAVip A metal-organic cage incorporating multiple light harvesting and catalytic centres for photochemical hydrogen production ????Nat Commun http://www.kidney.de/pget.php?&tw=1&pmid=27827376 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=27827376 #FOAvip English Wikipedia <ref>{{Cite pmid|27827376 }}</ref> A metal-organic cage incorporating multiple light harvesting and catalytic centres for photochemical hydrogen production #MMPMID27827376 Chen S ; Li K ; Zhao F ; Zhang L ; Pan M ; Fan YZ ; Guo J ; Shi J ; Su CY Nat Commun 2016[Nov]; 7 (ä): 13169 PMID27827376 show ga Photocatalytic water splitting is a natural but challenging chemical way of harnessing renewable solar power to generate clean hydrogen energy. Here we report a potential hydrogen-evolving photochemical molecular device based on a self-assembled ruthenium-palladium heterometallic coordination cage, incorporating multiple photo- and catalytic metal centres. The photophysical properties are investigated by absorption/emission spectroscopy, electrochemical measurements and preliminary DFT calculations and the stepwise electron transfer processes from ruthenium-photocentres to catalytic palladium-centres is probed by ultrafast transient absorption spectroscopy. The photocatalytic hydrogen production assessments reveal an initial reaction rate of 380??mol?h(-1) and a turnover number of 635 after 48?h. The efficient hydrogen production may derive from the directional electron transfers through multiple channels owing to proper organization of the photo- and catalytic multi-units within the octahedral cage, which may open a new door to design photochemical molecular devices with well-organized metallosupramolecules for homogenous photocatalytic applications. äA metal-organic cage incorporating multiple light harvesting and catal(epmc).pdf DeepDyve Pubget Overpricing