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10.1002/cphc.201500868 http://scihub22266oqcxt.onion/10.1002/cphc.201500868 C5086001!5086001!26693950     free     free     free Deprecated: Implicit conversion from float 209.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 209.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 209.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 209.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 209.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 209.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 243.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534       Chemphyschem 2016 ; 17 (5): 731-40 Nephropedia Template TP {{tp|p=26693950|t=2016. Role of the Inner Shell Architecture on Quantum Yield and Blinking Dynamics in Core/Multi-Shell Quantum Dots |pdf=|usr=}}{{26693950}} gab.com Text Role of the Inner Shell Architecture on Quantum Yield and Blinking Dynamics in Core/Multi-Shell Quantum Dots JO: Chemphyschem http://www.kidney.de/pget.php?&tw=1&pmid=26693950 #FOAvip Choosing the composition of the shell for QDs is not trivial, since both the band-edge energy offset and interfacial lattice mismatch play roles in influencing the final optical properties. One way to balance these competing effects is by forming multi-shells and/or gradient-alloyed shells. However, this introduces multiple interfaces and their relative effects on quantum yield and blinking are not yet fully understood. Here we undertake a systematic, comparative study of adding inner shells of single composition vs gradient-alloyed shells of cadmium/zinc chalogenides onto CdSe cores, and then capping with a thin ZnS outer shell to form various core/multi-shell configurations. We show that the inner shell architecture between the CdSe core and the outer ZnS shell plays a significant role in both quantum yield and blinking dynamics but that these effects are not correlated ? a high ensemble quantum yield doesn?t necessarily equate to reduced blinking. Two mathematical models have been proposed to describe the blinking dynamics ? the more common power-law model and a more recent multi-exponential model. By binning the same data with 1 ms and 20 ms resolution, we show that the on-times can be better described by the multi-exponential model while the off-times can be better described by the power-law model. We discuss physical mechanisms that might explain this behavior and how it can be affected by the inner shell architecture. Twit Text FOAVip Role of the Inner Shell Architecture on Quantum Yield and Blinking Dynamics in Core/Multi-Shell Quantum Dots ????Chemphyschem http://www.kidney.de/pget.php?&tw=1&pmid=26693950 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=26693950 #FOAvip English Wikipedia <ref>{{Cite pmid|26693950}}</ref> Role of the Inner Shell Architecture on Quantum Yield and Blinking Dynamics in Core/Multi-Shell Quantum Dots #MMPMID26693950 Bajwa P; Gao F; Nguyen A; Omogo B; Heyes CD Chemphyschem 2016[Mar]; 17 (5): 731-40 PMID26693950show ga Choosing the composition of the shell for QDs is not trivial, since both the band-edge energy offset and interfacial lattice mismatch play roles in influencing the final optical properties. One way to balance these competing effects is by forming multi-shells and/or gradient-alloyed shells. However, this introduces multiple interfaces and their relative effects on quantum yield and blinking are not yet fully understood. Here we undertake a systematic, comparative study of adding inner shells of single composition vs gradient-alloyed shells of cadmium/zinc chalogenides onto CdSe cores, and then capping with a thin ZnS outer shell to form various core/multi-shell configurations. We show that the inner shell architecture between the CdSe core and the outer ZnS shell plays a significant role in both quantum yield and blinking dynamics but that these effects are not correlated ? a high ensemble quantum yield doesn?t necessarily equate to reduced blinking. Two mathematical models have been proposed to describe the blinking dynamics ? the more common power-law model and a more recent multi-exponential model. By binning the same data with 1 ms and 20 ms resolution, we show that the on-times can be better described by the multi-exponential model while the off-times can be better described by the power-law model. We discuss physical mechanisms that might explain this behavior and how it can be affected by the inner shell architecture. äRole of the Inner Shell Architecture on Quantum Yield and Blinking Dyn(epmc).pdf DeepDyve Pubget Overpricing