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10.1021/acsomega.6b00076 http://scihub22266oqcxt.onion/10.1021/acsomega.6b00076 C5026461!5026461 !27656687     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=27656687 &cmd=llinks): Failed to open stream: HTTP request failed! 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Converting Light Energy to Chemical Energy: A New Catalytic Approach for Sustainable Environmental Remediation |pdf=|usr=}}{{27656687 }} gab.com Text Converting Light Energy to Chemical Energy: A New Catalytic Approach for Sustainable Environmental Remediation JO: ACS Omega http://www.kidney.de/pget.php?&tw=1&pmid=27656687 #FOAvip We report a synthetic approach to form cubic Cu(2)O/Pd composite structures and demonstrate their use as photocatalytic materials for tandem catalysis. Pd nanoparticles were deposited onto Cu(2)O cubes, and their tandem catalytic reactivity was studied via the reductive dehalogenation of polychlorinated biphenyls. The Pd content of the materials was gradually increased to examine its influence on particle morphology and catalytic performance. Materials were prepared at different Pd amounts and demonstrated a range of tandem catalytic reactivity. H(2) was generated via photocatalytic proton reduction initiated by Cu(2)O, followed by Pd-catalyzed dehalogenation using in situ generated H(2). The results indicate that material morphology and composition and substrate steric effects play important roles in controlling the overall reaction rate. Additionally, analysis of the postreacted materials revealed that a small number of the cubes had become hollow during the photodechlorination reaction. Such findings offer important insights regarding photocatalytic active sites and mechanisms, providing a pathway toward converting light-based energy to chemical energy for sustainable catalytic reactions not typically driven via light. Twit Text FOAVip Converting Light Energy to Chemical Energy: A New Catalytic Approach for Sustainable Environmental Remediation ????ACS Omega http://www.kidney.de/pget.php?&tw=1&pmid=27656687 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=27656687 #FOAvip English Wikipedia <ref>{{Cite pmid|27656687 }}</ref> Converting Light Energy to Chemical Energy: A New Catalytic Approach for Sustainable Environmental Remediation #MMPMID27656687 Nguyen MA ; Zahran EM ; Wilbon AS ; Besmer AV ; Cendan VJ ; Ranson WA ; Lawrence RL ; Cohn JL ; Bachas LG ; Knecht MR ACS Omega 2016[Jul]; 1 (1 ): 41-51 PMID27656687 show ga We report a synthetic approach to form cubic Cu(2)O/Pd composite structures and demonstrate their use as photocatalytic materials for tandem catalysis. Pd nanoparticles were deposited onto Cu(2)O cubes, and their tandem catalytic reactivity was studied via the reductive dehalogenation of polychlorinated biphenyls. The Pd content of the materials was gradually increased to examine its influence on particle morphology and catalytic performance. Materials were prepared at different Pd amounts and demonstrated a range of tandem catalytic reactivity. H(2) was generated via photocatalytic proton reduction initiated by Cu(2)O, followed by Pd-catalyzed dehalogenation using in situ generated H(2). The results indicate that material morphology and composition and substrate steric effects play important roles in controlling the overall reaction rate. Additionally, analysis of the postreacted materials revealed that a small number of the cubes had become hollow during the photodechlorination reaction. Such findings offer important insights regarding photocatalytic active sites and mechanisms, providing a pathway toward converting light-based energy to chemical energy for sustainable catalytic reactions not typically driven via light. äConverting Light Energy to Chemical Energy: A New Catalytic Approach f(epmc).pdf DeepDyve Pubget Overpricing