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10.1063/1.4947098

http://scihub22266oqcxt.onion/10.1063/1.4947098
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C4841798!4841798!27158637
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suck abstract from ncbi


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pmid27158637      Struct+Dyn 2016 ; 3 (2): ä
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  • Femtosecond few- to single-electron point-projection microscopy for nanoscale dynamic imaging #MMPMID27158637
  • Bainbridge AR; Barlow Myers CW; Bryan WA
  • Struct Dyn 2016[Mar]; 3 (2): ä PMID27158637show ga
  • Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron per pulse. Here, we demonstrate femtosecond single-electron point projection microscopy (fs-ePPM) in a laser-pump fs-e-probe configuration. The electrons have an energy of only 150?eV and take tens of picoseconds to propagate to the object under study. Nonetheless, we achieve a temporal resolution with a standard deviation of 114?fs (equivalent to a full-width at half-maximum of 269?±?40?fs) combined with a spatial resolution of 100?nm, applied to a localized region of charge at the apex of a nanoscale metal tip induced by 30?fs 800?nm laser pulses at 50?kHz. These observations demonstrate real-space imaging of reversible processes, such as tracking charge distributions, is feasible whilst maintaining femtosecond resolution. Our findings could find application as a characterization method, which, depending on geometry, could resolve tens of femtoseconds and tens of nanometres. Dynamically imaging electric and magnetic fields and charge distributions on sub-micron length scales opens new avenues of ultrafast dynamics. Furthermore, through the use of active compression, such pulses are an ideal seed for few-femtosecond to attosecond imaging applications which will access sub-optical cycle processes in nanoplasmonics.
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