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10.1038/srep12045 http://scihub22266oqcxt.onion/10.1038/srep12045 C4496785!4496785 !26155988     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=26155988 &cmd=llinks): Failed to open stream: HTTP request failed! 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In-situ observation for growth of hierarchical metal-organic frameworks and their self-sequestering mechanism for gas storage |pdf=|usr=}}{{26155988 }} gab.com Text In-situ observation for growth of hierarchical metal-organic frameworks and their self-sequestering mechanism for gas storage JO: Sci Rep http://www.kidney.de/pget.php?&tw=1&pmid=26155988 #FOAvip Although structures with the single functional constructions and micropores were demonstrated to capture many different molecules such as carbon dioxide, methane, and hydrogen with high capacities at low temperatures, their feeble interactions still limit practical applications at room temperature. Herein, we report in-situ growth observation of hierarchical pores in pomegranate metal-organic frameworks (pmg-MOFs) and their self-sequestering storage mechanism, not observed for pristine MOFs. Direct observation of hierarchical pores inside the pmg-MOF was evident by in-situ growth X-ray measurements while self-sequestering storage mechanism was revealed by in-situ gas sorption X-ray analysis and molecular dynamics simulations. The results show that meso/macropores are created at the early stage of crystal growth and then enclosed by micropore crystalline shells, where hierarchical pores are networking under self-sequestering mechanism to give enhanced gas storage. This pmg-MOF gives higher CO2 (39%) and CH4 (14%) storage capacity than pristine MOF at room temperature, in addition to fast kinetics with robust capacity retention during gas sorption cycles, thus giving the clue to control dynamic behaviors of gas adsorption. Twit Text FOAVip In-situ observation for growth of hierarchical metal-organic frameworks and their self-sequestering mechanism for gas storage ????Sci Rep http://www.kidney.de/pget.php?&tw=1&pmid=26155988 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=26155988 #FOAvip English Wikipedia <ref>{{Cite pmid|26155988 }}</ref> In-situ observation for growth of hierarchical metal-organic frameworks and their self-sequestering mechanism for gas storage #MMPMID26155988 Hyo Park J ; Choi KM ; Jeon HJ ; Jung Choi Y ; Kang JK Sci Rep 2015[Jul]; 5 (ä): 12045 PMID26155988 show ga Although structures with the single functional constructions and micropores were demonstrated to capture many different molecules such as carbon dioxide, methane, and hydrogen with high capacities at low temperatures, their feeble interactions still limit practical applications at room temperature. Herein, we report in-situ growth observation of hierarchical pores in pomegranate metal-organic frameworks (pmg-MOFs) and their self-sequestering storage mechanism, not observed for pristine MOFs. Direct observation of hierarchical pores inside the pmg-MOF was evident by in-situ growth X-ray measurements while self-sequestering storage mechanism was revealed by in-situ gas sorption X-ray analysis and molecular dynamics simulations. The results show that meso/macropores are created at the early stage of crystal growth and then enclosed by micropore crystalline shells, where hierarchical pores are networking under self-sequestering mechanism to give enhanced gas storage. This pmg-MOF gives higher CO2 (39%) and CH4 (14%) storage capacity than pristine MOF at room temperature, in addition to fast kinetics with robust capacity retention during gas sorption cycles, thus giving the clue to control dynamic behaviors of gas adsorption. äIn-situ observation for growth of hierarchical metal-organic framework(epmc).pdf DeepDyve Pubget Overpricing