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10.1073/pnas.1420734111 http://scihub22266oqcxt.onion/10.1073/pnas.1420734111 C4280589!4280589!25489068     free     free     free Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 267.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534       Proc+Natl+Acad+Sci+U+S+A 2014 ; 111 (51): 18132-7 Nephropedia Template TP {{tp|p=25489068|t=2014. Site-specific vibrational spectral signatures of water molecules in the magic H3O+(H2O)20 and Cs+(H2O)20 clusters |pdf=|usr=}}{{25489068}} gab.com Text Site-specific vibrational spectral signatures of water molecules in the magic H3O+(H2O)20 and Cs+(H2O)20 clusters JO: Proc Natl Acad Sci U S A http://www.kidney.de/pget.php?&tw=1&pmid=25489068 #FOAvip Understanding the mechanics underlying the diffuse OH stretching spectrum of water is a grand challenge for contemporary physical chemistry. Water clusters play an increasingly important role in this endeavor, as they allow one to freeze and isolate the spectral behavior of relatively large assemblies with well-defined network morphologies. We exploit recently developed, hybrid instruments that integrate laser spectroscopy with cryogenic ion trap mass spectrometry to capture the H3O+ and Cs+ ions in cage structures formed by 20 water molecules. Their infrared spectra reveal a pattern of distinct transitions that is unprecedented for water networks in this size range. Theoretical analysis of these patterns then reveals the intramolecular distortions associated with water molecules at various sites in the 3D cages. Twit Text FOAVip Site-specific vibrational spectral signatures of water molecules in the magic H3O+(H2O)20 and Cs+(H2O)20 clusters ????Proc Natl Acad Sci U S A http://www.kidney.de/pget.php?&tw=1&pmid=25489068 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=25489068 #FOAvip English Wikipedia <ref>{{Cite pmid|25489068}}</ref> Site-specific vibrational spectral signatures of water molecules in the magic H3O+(H2O)20 and Cs+(H2O)20 clusters #MMPMID25489068 Fournier JA; Wolke CT; Johnson CJ; Johnson MA; Heine N; Gewinner S; Schöllkopf W; Esser TK; Fagiani MR; Knorke H; Asmis KR Proc Natl Acad Sci U S A 2014[Dec]; 111 (51): 18132-7 PMID25489068show ga Understanding the mechanics underlying the diffuse OH stretching spectrum of water is a grand challenge for contemporary physical chemistry. Water clusters play an increasingly important role in this endeavor, as they allow one to freeze and isolate the spectral behavior of relatively large assemblies with well-defined network morphologies. We exploit recently developed, hybrid instruments that integrate laser spectroscopy with cryogenic ion trap mass spectrometry to capture the H3O+ and Cs+ ions in cage structures formed by 20 water molecules. Their infrared spectra reveal a pattern of distinct transitions that is unprecedented for water networks in this size range. Theoretical analysis of these patterns then reveals the intramolecular distortions associated with water molecules at various sites in the 3D cages. äSite-specific vibrational spectral signatures of water molecules in th(epmc).pdf DeepDyve Pubget Overpricing