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10.1002/smll.202509917 http://scihub22266oqcxt.onion/10.1002/smll.202509917 41319320!?!41319320 Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=41319320&cmd=llinks): Failed to open stream: HTTP request failed! HTTP/1.1 429 Too Many Requests in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 215       Small 2025 ; ? (?): e09917 Nephropedia Template TP {{tp|p=41319320|t=2025. Highly Conductive and Supertough PVDF-Based Electrolytes with Self-Defective Fillers for Solid-State Lithium Metal Batteries |pdf=|usr=}}{{41319320}} gab.com Text Highly Conductive and Supertough PVDF-Based Electrolytes with Self-Defective Fillers for Solid-State Lithium Metal Batteries JO: Small http://www.kidney.de/pget.php?&tw=1&pmid=41319320 #FOAvip Advanced PVDF-based electrolytes with ceramic-like ion migration behavior, near-separator-level toughness, and excellent oxidation resistance are critical for the practical implementation of solid-state lithium-metal batteries (SSLMBs). However, the superior ion conductivity, robust mechanical property, and wide electrochemical stability usually cannot be achieved simultaneously. Herein, the self-defective silicon (Si) fillers with silicon/silicon oxide (Si/SiO(x),0<x</=2) heterogeneous interfaces are doped into the PVDF matrix to construct the highly conductive and supertough PVDF-based electrolytes. Results reveal that the self-defective Si will spontaneously participate in the Li(+)-solvation state and convert all solvation structure into the Li(+)-[solvent](x)-[anion](y) (x</=y) configuration. The anion-rich Li(+) coordination environment not only accelerate Li(+) diffusion rate but also promotes the formation of the anion-dominated bilayer interphase. Meanwhile, the strong Lewis acid-base interaction of PVDF/SiO(x) interface effectively suppresses phase separation initiated by uneven solvent evaporation. Benefiting from the modified Li(+) transport environment and phase regulation, the obtained electrolytes exhibit impressive comprehensive properties, including ionic conductivity of 0.44 mS cm(-1), tensile strength of 16.5 Mpa, and voltage window of 5.07 V. Besides, the Li||Li symmetrical batteries present outstanding cycling under the current density of 0.1 mA cm(-2) (>6200 h), and the LFP||Li batteries exhibit remarkable fast-charging behavior at 10 C with the capacity retention of 82.29%. Twit Text FOAVip Highly Conductive and Supertough PVDF-Based Electrolytes with Self-Defective Fillers for Solid-State Lithium Metal Batteries ????Small http://www.kidney.de/pget.php?&tw=1&pmid=41319320 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=41319320 #FOAvip English Wikipedia <ref>{{Cite pmid|41319320}}</ref> Highly Conductive and Supertough PVDF-Based Electrolytes with Self-Defective Fillers for Solid-State Lithium Metal Batteries #MMPMID41319320 Fan K; Wang B; Chen J; Cao K; Zhang C; Chen J; Zhao Y; Yuan J; Hu Z; Wang L Small 2025[Nov]; ? (?): e09917 PMID41319320show ga Advanced PVDF-based electrolytes with ceramic-like ion migration behavior, near-separator-level toughness, and excellent oxidation resistance are critical for the practical implementation of solid-state lithium-metal batteries (SSLMBs). However, the superior ion conductivity, robust mechanical property, and wide electrochemical stability usually cannot be achieved simultaneously. Herein, the self-defective silicon (Si) fillers with silicon/silicon oxide (Si/SiO(x),06200 h), and the LFP||Li batteries exhibit remarkable fast-charging behavior at 10 C with the capacity retention of 82.29%. ?Highly Conductive and Supertough PVDF-Based Electrolytes with Self-Def(epmc).pdf DeepDyve Pubget Overpricing