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10.1021/acsami.5c09311 http://scihub22266oqcxt.onion/10.1021/acsami.5c09311 40590122!ä!40590122 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 229.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 263.2 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Warning: imagejpeg(C:\Inetpub\vhosts\kidney.de\httpdocs\phplern\40590122.jpg): Failed to open stream: No such file or directory in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 117       ACS+Appl+Mater+Interfaces 2025 ; ä (ä): ä Nephropedia Template TP {{tp|p=40590122|t=2025. Ionic Liquid-Functionalized Covalent Organic Frameworks for CO(2) to Cyclic Carbonate Conversion under Solvent, Metal, and Co-Catalyst Free Conditions |pdf=|usr=}}{{40590122}} gab.com Text Ionic Liquid-Functionalized Covalent Organic Frameworks for CO(2) to Cyclic Carbonate Conversion under Solvent, Metal, and Co-Catalyst Free Conditions JO: ACS Appl Mater Interfaces http://www.kidney.de/pget.php?&tw=1&pmid=40590122 #FOAvip The efficient and sustainable conversion of carbon dioxide (CO(2)) into value-added chemicals represents a promising approach for addressing environmental and energy challenges. Herein, we report the design and synthesis of a series of ionic liquid-functionalized covalent organic frameworks, [DD](X%)-PB-COF (X = 25, 50, 75, 100), via postsynthetic modification of hydroxyl-containing COFs using triethylenediamine-based ionic liquids. The resulting materials exhibit high crystallinity, tunable active site density, and well-defined one-dimensional channels conducive to CO(2) mass transport. Among the series, [DD](75%)-PB-COF showed the highest catalytic activity for the cycloaddition of CO(2) with epoxides under metal-free, solvent-free, cocatalyst-free, and pressure-free conditions, affording cyclic carbonates in excellent yields with >99% selectivity. The catalyst demonstrated broad substrate scope, including aliphatic, aromatic, and functionalized epoxides, and retained its activity and structural integrity over multiple recycling cycles. Mechanistic studies and in situ IR analysis revealed a synergistic dual-center catalytic mode, involving both electrophilic activation and nucleophilic ring-opening, enabled by the ionic liquid moieties and the COF architecture. This work presents a robust and recyclable heterogeneous catalyst platform for green CO(2) fixation, offering new insights into the integration of ionic liquids and crystalline porous frameworks for sustainable catalysis. Twit Text FOAVip Ionic Liquid-Functionalized Covalent Organic Frameworks for CO(2) to Cyclic Carbonate Conversion under Solvent, Metal, and Co-Catalyst Free Conditions ????ACS Appl Mater Interfaces http://www.kidney.de/pget.php?&tw=1&pmid=40590122 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=40590122 #FOAvip English Wikipedia <ref>{{Cite pmid|40590122}}</ref> Ionic Liquid-Functionalized Covalent Organic Frameworks for CO(2) to Cyclic Carbonate Conversion under Solvent, Metal, and Co-Catalyst Free Conditions #MMPMID40590122 Wen TT; Liu XH; Feng JR; Zheng SY; Zhong HK; Zhang HW; Xue C; Zhou XT ACS Appl Mater Interfaces 2025[Jul]; ä (ä): ä PMID40590122show ga The efficient and sustainable conversion of carbon dioxide (CO(2)) into value-added chemicals represents a promising approach for addressing environmental and energy challenges. Herein, we report the design and synthesis of a series of ionic liquid-functionalized covalent organic frameworks, [DD](X%)-PB-COF (X = 25, 50, 75, 100), via postsynthetic modification of hydroxyl-containing COFs using triethylenediamine-based ionic liquids. The resulting materials exhibit high crystallinity, tunable active site density, and well-defined one-dimensional channels conducive to CO(2) mass transport. Among the series, [DD](75%)-PB-COF showed the highest catalytic activity for the cycloaddition of CO(2) with epoxides under metal-free, solvent-free, cocatalyst-free, and pressure-free conditions, affording cyclic carbonates in excellent yields with >99% selectivity. The catalyst demonstrated broad substrate scope, including aliphatic, aromatic, and functionalized epoxides, and retained its activity and structural integrity over multiple recycling cycles. Mechanistic studies and in situ IR analysis revealed a synergistic dual-center catalytic mode, involving both electrophilic activation and nucleophilic ring-opening, enabled by the ionic liquid moieties and the COF architecture. This work presents a robust and recyclable heterogeneous catalyst platform for green CO(2) fixation, offering new insights into the integration of ionic liquids and crystalline porous frameworks for sustainable catalysis. äIonic Liquid-Functionalized Covalent Organic Frameworks for CO(2) to C(epmc).pdf DeepDyve Pubget Overpricing