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10.1038/ncomms12312 http://scihub22266oqcxt.onion/10.1038/ncomms12312 C4992055!4992055 !27531582     free     free     free Warning: file_get_contents(https://eutils.ncbi.nlm.nih.gov/entrez/eutils/elink.fcgi?dbfrom=pubmed&id=27531582 &cmd=llinks): Failed to open stream: HTTP request failed! HTTP/1.1 429 Too Many Requests in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 215 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Deprecated: Implicit conversion from float 233.6 to int loses precision in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 534 Warning: imagejpeg(C:\Inetpub\vhosts\kidney.de\httpdocs\phplern\27531582 .jpg): Failed to open stream: No such file or directory in C:\Inetpub\vhosts\kidney.de\httpdocs\pget.php on line 117       Nat+Commun 2016 ; 7 (ä): 12312 Nephropedia Template TP {{tp|p=27531582 |t=2016. Spectroscopic and computational investigation of actinium coordination chemistry |pdf=|usr=}}{{27531582 }} gab.com Text Spectroscopic and computational investigation of actinium coordination chemistry JO: Nat Commun http://www.kidney.de/pget.php?&tw=1&pmid=27531582 #FOAvip Actinium-225 is a promising isotope for targeted-? therapy. Unfortunately, progress in developing chelators for medicinal applications has been hindered by a limited understanding of actinium chemistry. This knowledge gap is primarily associated with handling actinium, as it is highly radioactive and in short supply. Hence, Ac(III) reactivity is often inferred from the lanthanides and minor actinides (that is, Am, Cm), with limited success. Here we overcome these challenges and characterize actinium in HCl solutions using X-ray absorption spectroscopy and molecular dynamics density functional theory. The Ac-Cl and Ac-OH2O distances are measured to be 2.95(3) and 2.59(3) Å, respectively. The X-ray absorption spectroscopy comparisons between Ac(III) and Am(III) in HCl solutions indicate Ac(III) coordinates more inner-sphere Cl(1-) ligands (3.2±1.1) than Am(III) (0.8±0.3). These results imply diverse reactivity for the +3 actinides and highlight the unexpected and unique Ac(III) chemical behaviour. Twit Text FOAVip Spectroscopic and computational investigation of actinium coordination chemistry ????Nat Commun http://www.kidney.de/pget.php?&tw=1&pmid=27531582 #FOAvip Twit Text # Free Paper on # # # # # LINK http://www.kidney.de/pget.php?&tw=1&pmid=27531582 #FOAvip English Wikipedia <ref>{{Cite pmid|27531582 }}</ref> Spectroscopic and computational investigation of actinium coordination chemistry #MMPMID27531582 Ferrier MG ; Batista ER ; Berg JM ; Birnbaum ER ; Cross JN ; Engle JW ; La Pierre HS ; Kozimor SA ; Lezama Pacheco JS ; Stein BW ; Stieber SC ; Wilson JJ Nat Commun 2016[Aug]; 7 (ä): 12312 PMID27531582 show ga Actinium-225 is a promising isotope for targeted-? therapy. Unfortunately, progress in developing chelators for medicinal applications has been hindered by a limited understanding of actinium chemistry. This knowledge gap is primarily associated with handling actinium, as it is highly radioactive and in short supply. Hence, Ac(III) reactivity is often inferred from the lanthanides and minor actinides (that is, Am, Cm), with limited success. Here we overcome these challenges and characterize actinium in HCl solutions using X-ray absorption spectroscopy and molecular dynamics density functional theory. The Ac-Cl and Ac-OH2O distances are measured to be 2.95(3) and 2.59(3) Å, respectively. The X-ray absorption spectroscopy comparisons between Ac(III) and Am(III) in HCl solutions indicate Ac(III) coordinates more inner-sphere Cl(1-) ligands (3.2±1.1) than Am(III) (0.8±0.3). These results imply diverse reactivity for the +3 actinides and highlight the unexpected and unique Ac(III) chemical behaviour. |*Models, Molecular [MESH] |*X-Ray Absorption Spectroscopy [MESH] |Actinium/*chemistry [MESH] |Fourier Analysis [MESH] |Radioisotopes [MESH]Spectroscopic and computational investigation of actinium coordination(epmc).pdf DeepDyve Pubget Overpricing