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10.1073/pnas.1615281113

http://scihub22266oqcxt.onion/10.1073/pnas.1615281113
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suck abstract from ncbi


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pmid27911819
      Proc+Natl+Acad+Sci+U+S+A 2016 ; 113 (50 ): 14201-14206
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  • Programmable and reversible plasmon mode engineering #MMPMID27911819
  • Yang A ; Hryn AJ ; Bourgeois MR ; Lee WK ; Hu J ; Schatz GC ; Odom TW
  • Proc Natl Acad Sci U S A 2016[Dec]; 113 (50 ): 14201-14206 PMID27911819 show ga
  • Plasmonic nanostructures with enhanced localized optical fields as well as narrow linewidths have driven advances in numerous applications. However, the active engineering of ultranarrow resonances across the visible regime-and within a single system-has not yet been demonstrated. This paper describes how aluminum nanoparticle arrays embedded in an elastomeric slab may exhibit high-quality resonances with linewidths as narrow as 3 nm at wavelengths not accessible by conventional plasmonic materials. We exploited stretching to improve and tune simultaneously the optical response of as-fabricated nanoparticle arrays by shifting the diffraction mode relative to single-particle dipolar or quadrupolar resonances. This dynamic modulation of particle-particle spacing enabled either dipolar or quadrupolar lattice modes to be selectively accessed and individually optimized. Programmable plasmon modes offer a robust way to achieve real-time tunable materials for plasmon-enhanced molecular sensing and plasmonic nanolasers and opens new possibilities for integrating with flexible electronics.
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